Topological transport in monolayer jacutingaite

Muzamil Shah, Muhammad Sabieh Anwar

Published 2024-12-22Version 1

Monolayer-jacutingaite (Pt2HgSe3) has been predicted to be the first large-gap Kane-Mele quantum spin Hall insulator. Materials in the jacutingaite family undergo topological phase transitions (TPTs), i.e., from a topologically non-trivial to a semimetallic phase and further to the normal insulating phase when exposed to electric fields and off-resonance, high-frequency and high-intensity laser irradiation. In this article, we investigate the rich tapestry of topological phases in this unique material in the presence of an appropriate choice of off-resonance circularly polarized laser fields and staggered sublattice potentials. The interplay of these stimuli with large spin-orbit coupling, due to the buckled structure of jacutingaite materials, results in the emergence of quantum spin Hall insulator, valley-spin-polarized metal, spin-polarized metal, photo-induced quantum Hall insulator, anomalous quantum Hall insulator and band insulator phases. By analyzing the band structures, we compute Berry curvatures in different topological regimes for the $K$ and $K'$ valleys. Furthermore, by using the Kubo formula, we calculate the spin-valley resolved longitudinal and Hall conductivities as a function of photon energies showing that the conductivities exhibit a strong topological state dependence. The photon energy of the intraband and interband optical transitions can be tuned by varying the electric and optical fields. Finally, we demonstrate that by modulating the chemical potential, some of the allowed optical transitions become Pauli blocked due to the optical selection rules