Observation of Chern insulator in crystalline ABCA-tetralayer graphene with spin-orbit coupling

Yating Sha, Jian Zheng, Kai Liu, Hong Du, Kenji Watanabe, Takashi Taniguchi, Jinfeng Jia, Zhiwen Shi, Ruidan Zhong, Guorui Chen

Published 2023-10-27Version 1

Degeneracies in multilayer graphene, including spin, valley, and layer degrees of freedom, are susceptible to Coulomb interactions and can result into rich broken-symmetry states. In this work, we report a ferromagnetic state in charge neutral ABCA-tetralayer graphene driven by proximity-induced spin-orbit coupling from adjacent WSe2. The ferromagnetic state is further identified as a Chern insulator with Chern number of 4, and its Hall resistance reaches 78% and 100% quantization of h/4e2 at zero and 0.4 tesla, respectively. Three broken-symmetry insulating states, layer-antiferromagnet, Chern insulator and layer-polarized insulator and their transitions can be continuously tuned by the vertical displacement field. Remarkably, the magnetic order of the Chern insulator can be switched by three knobs, including magnetic field, electrical doping, and vertical displacement field.