Microscopic theory of cavity-enhanced interactions of dipolaritons

Esben R. Christensen, Arturo Camacho-Guardian, Ovidiu Cotlet, Atac Imamoglu, Michiel Wouters, Georg M. Bruun, Iacopo Carusotto

Published 2022-12-05Version 1

We develop a theoretical model for the interaction strength between a pair of exciton-polaritons with finite and parallel static electric-dipole moments. In stark contrast to simple perturbative arguments predicting the interaction to be reduced due to the hybridisation with cavity photons, we find that the strong coupling to a cavity mode leads to a drastic enhancement of the polariton interactions as compared to bare excitons. This enhancement is caused by the small polariton mass due to its photonic component, which increases the kinetic cost associated with minimising the dipole-dipole repulsion. Microscopic numerical calculations for one-dimensional geometries show that the interaction strength for the lower polariton branch is maximal when the exciton and the cavity mode are close to resonance, and can easily exceed state-of-the-art cavity decay rates for realistic confinement lengths, thus entering the polariton blockade regime. Analytical extension of our results to two-dimensional polariton systems highlight dipolar polaritons as a most promising solid-state platform to realize strongly interacting photonic systems.