Spectrally Selective Thermal Emission from Graphene Decorated with Metallic Nanoparticles

Jayden Craft, Muhammad Waqas Shabbir, Dirk R. Englund, Richard M. Osgood III, Michael N. Leuenberger

Published 2022-09-23Version 1

We showed in past work that nanopatterned monolayer graphene (NPG) enables spectrally selective thermal emission in the mid-infrared (mid-IR) from 3 to 12 $\mu$m. In that case the spectral selection is realized by means of the localized surface plasmon (LSP) resonances inside graphene. Here we show that graphene decorated with metallic nanoparticles, such as Ag nanocubes or nanospheres, also realize spectrally selective thermal emission, but in this case by means of acoustic graphene plasmons (AGPs) localized between graphene and the Ag nanoparticle inside a dielectric material. Our finite-difference time domain (FDTD) calculations show that the spectrally selective thermal radiation emission can be tuned by means of a gate voltage into two different wavelength regimes, namely the atmospherically opaque regime between $\lambda=5$ $\mu$m and $\lambda=8$ $\mu$m or the atmospherically transparent regime between $\lambda=8$ $\mu$m and $\lambda=12$ $\mu$m. This allows for electric switching between radiative heat trapping mode for the fomer regime and radiative cooling mode for the latter regime. Our theoretical results can be used to develop graphene-based thermal management systems for smart fabrics.