Spatiotemporal intermittency and localized dynamic fluctuations upon approaching the glass transition

J. Ariel Rodriguez Fris, Eric R. Weeks, Francesco Sciortino, Gustavo A. Appignanesi

Published 2018-01-30Version 1

We introduce a new and robust approach for characterizing spatially and temporally heterogeneous behavior within a system based on the evolution of dynamic fuctuations once averaged over different space lengths and time scales. We apply it to investigate the dynamics in two canonical systems as the glass transition is approached: simulated Lennard-Jones liquids and experimental dense colloidal suspensions. We find that in both cases the onset of glassines is marked by spatially localized dynamic fluctuations originating in regions of correlated mobile particles. By removing the trivial system size dependence of the fluctuations we show that such regions contain tens to hundreds of particles for time scales corresponding to maximally non-Gaussian dynamics.