{ "id": "cond-mat/0607447", "version": "v1", "published": "2006-07-18T12:56:46.000Z", "updated": "2006-07-18T12:56:46.000Z", "title": "Vibrationally Induced Two-Level Systems in Single-Molecule Junctions", "authors": [ "W. H. A. Thijssen", "D. Djukic", "A. F. Otte", "R. H. Bremmer", "J. M. van Ruitenbeek" ], "comment": "4 pages, 4 figures", "doi": "10.1103/PhysRevLett.97.226806", "categories": [ "cond-mat.mes-hall" ], "abstract": "Single-molecule junctions are found to show anomalous spikes in dI/dV spectra. The position in energy of the spikes are related to local vibration mode energies. A model of vibrationally induced two-level systems reproduces the data very well. This mechanism is expected to be quite general for single-molecule junctions. It acts as an intrinsic amplification mechanism for local vibration mode features and may be exploited as a new spectroscopic tool.", "revisions": [ { "version": "v1", "updated": "2006-07-18T12:56:46.000Z" } ], "analyses": { "keywords": [ "single-molecule junctions", "local vibration mode features", "local vibration mode energies", "intrinsic amplification mechanism", "vibrationally induced two-level systems reproduces" ], "tags": [ "journal article" ], "publication": { "publisher": "APS", "journal": "Phys. Rev. Lett." }, "note": { "typesetting": "TeX", "pages": 4, "language": "en", "license": "arXiv", "status": "editable" } } }