{ "id": "cond-mat/0211562", "version": "v1", "published": "2002-11-25T17:34:53.000Z", "updated": "2002-11-25T17:34:53.000Z", "title": "Single-File Diffusion of Atomic and Colloidal Systems: Asymptotic Laws", "authors": [ "Markus Kollmann" ], "comment": "4 pages", "doi": "10.1103/PhysRevLett.90.180602", "categories": [ "cond-mat.stat-mech", "cond-mat.soft" ], "abstract": "In this work we present a general derivation of the non-Fickian behavior for the self-diffusion of identically interacting particle systems with excluded mutual passage. We show that the conditional probability distribution of finding a particle at position $x_{t}$ after time $t$, when the particle was located at $x_{0}$ at $t=0$, follows a Gaussian distribution in the long-time limit, with variance $2W(t)\\sim t^{1/2}$ for overdamped systems and with variance $2W(t)\\sim t$ for classical systems. The asymptotic behavior of the mean-squared displacement, $W(t)$, is shown to be independent of the nature of interactions for homogeneous systems in the fluid state. Moreover, the long-time behavior of self-diffusion is determined by short-time and large scale collective density fluctuations.", "revisions": [ { "version": "v1", "updated": "2002-11-25T17:34:53.000Z" } ], "analyses": { "keywords": [ "colloidal systems", "asymptotic laws", "single-file diffusion", "large scale collective density fluctuations", "conditional probability distribution" ], "tags": [ "journal article" ], "publication": { "publisher": "APS", "journal": "Phys. Rev. Lett." }, "note": { "typesetting": "TeX", "pages": 4, "language": "en", "license": "arXiv", "status": "editable" } } }