{ "id": "2502.08546", "version": "v1", "published": "2025-02-12T16:29:16.000Z", "updated": "2025-02-12T16:29:16.000Z", "title": "Monolayer transition metal dichalcogenides under finite-pulse polarized radiation", "authors": [ "Alejandro S. Gómez", "Yuriko Baba", "Francisco Domínguez-Adame", "Rafael A. Molina" ], "comment": "17 pages, 12 figures", "categories": [ "cond-mat.mes-hall", "cond-mat.other" ], "abstract": "Recent advances in time-resolved angle-resolved photoemission spectroscopy have enabled access to ultrafast electron states and their spin dynamics in solids. Atomically thin transition metal dichalcogenides are paradigmatic two-dimensional materials where electron momentum and spin degrees of freedom are coupled, being suitable candidates for time-resolved spectroscopy studies. In this work, we present a thorough study of the electron dynamics when these materials are subject to an intense finite-pulse driving radiation. We extend the scope of the conventional Floquet engineering and rely of the so-called $t-t^{\\prime}$ formalism to deal with driving fields described with two distinct time scales, namely the envelope amplitude timescale and the time period of the external field. The interplay between the finite-pulse timescales and the intrinsic properties of the electrons gives rise to transient valley polarization and dynamical modifications of band structures, revealed by the time-dependent circular dichroism of the sample.", "revisions": [ { "version": "v1", "updated": "2025-02-12T16:29:16.000Z" } ], "analyses": { "keywords": [ "monolayer transition metal dichalcogenides", "finite-pulse polarized radiation", "atomically thin transition metal dichalcogenides", "ultrafast electron states", "intense finite-pulse driving radiation" ], "note": { "typesetting": "TeX", "pages": 17, "language": "en", "license": "arXiv", "status": "editable" } } }