{ "id": "2309.12131", "version": "v1", "published": "2023-09-21T14:52:04.000Z", "updated": "2023-09-21T14:52:04.000Z", "title": "Temperature dependence of charge conversion during NV-center relaxometry", "authors": [ "Isabel Cardoso Barbosa", "Jonas Gutsche", "Dennis Lönard", "Stefan Dix", "Artur Widera" ], "comment": "8 pages, 7 figures", "categories": [ "quant-ph", "cond-mat.mes-hall" ], "abstract": "Temperature-dependent nitrogen-vacancy (NV)-center relaxometry is an established tool to characterize paramagnetic molecules near to a sensing diamond, gaining momentum in different fields of science. However, recent results indicate that conversion between NV-center charge states impedes these measurements and influences the results for the $T_1$ time. While the temperature dependence of NV centers' $T_1$ time is well-studied, additional contributions from temperature-dependent charge conversion during the dark time may further affect the measurement results. We combine temperature-dependent relaxometry and fluorescence spectroscopy at varying laser powers to unravel the temperature dependence of charge conversion in nanodiamond for biologically relevant temperatures. While we observe a decrease of the $T_1$ time with increasing temperatures, charge conversion remains unaffected by the temperature change. These results allow the temperature dependent performance of $T_1$ relaxometry without further consideration of temperature dependence of charge conversion.", "revisions": [ { "version": "v1", "updated": "2023-09-21T14:52:04.000Z" } ], "analyses": { "keywords": [ "temperature dependence", "nv-center relaxometry", "nv-center charge states impedes", "temperature-dependent charge conversion", "charge conversion remains" ], "note": { "typesetting": "TeX", "pages": 8, "language": "en", "license": "arXiv", "status": "editable" } } }