{ "id": "2204.11498", "version": "v1", "published": "2022-04-25T08:27:26.000Z", "updated": "2022-04-25T08:27:26.000Z", "title": "Reduced effective magnetization and damping by slowly-relaxing impurities in strained $γ$-$\\mathrm{Fe_2O_3}$ thin films", "authors": [ "Manuel Müller", "Monika Scheufele", "Janine Gückelhorn", "Luis Flacke", "Mathias Weiler", "Hans Huebl", "Stephan Geprägs", "Rudolf Gross", "Matthias Althammer" ], "comment": "10 pages, 8 figures", "categories": [ "cond-mat.mes-hall" ], "abstract": "We study the static and dynamic magnetic properties of epitaxially strained $\\gamma$-$\\mathrm{Fe_2O_3}$ (maghemite) thin films grown via pulsed-laser deposition on MgO substrates by SQUID magnetometry and cryogenic broadband ferromagnetic resonance experiments. SQUID magnetometry measurements reveal hysteretic magnetization curves for magnetic fields applied both in- and out of the sample plane. From the magnetization dynamics of our thin films, we find a small negative effective magnetization in agreement with a strain induced perpendicular magnetic anisotropy. Moreover, we observe a non-linear evolution of the ferromagnetic resonance-linewidth as function of the microwave frequency and explain this finding with a model based on slowly relaxing impurities, the so-called slow relaxor model. By investigating the magnetization dynamics in our maghemite thin films as a function of frequency and temperature, we can isolate the temperature dependent contribution of the slowly relaxing impurities to the resonance linewidth and, in particular, observe a sign change in the effective magnetization. This finding provides evidence for a transition of the magnetic anisotropy from a perpendicular easy axis to an easy in-plane anisotropy for reduced temperatures.", "revisions": [ { "version": "v1", "updated": "2022-04-25T08:27:26.000Z" } ], "analyses": { "keywords": [ "thin films", "reduced effective magnetization", "broadband ferromagnetic resonance experiments", "magnetometry measurements reveal hysteretic", "slowly-relaxing impurities" ], "note": { "typesetting": "TeX", "pages": 10, "language": "en", "license": "arXiv", "status": "editable" } } }