{ "id": "2204.01025", "version": "v1", "published": "2022-04-03T08:19:56.000Z", "updated": "2022-04-03T08:19:56.000Z", "title": "Trion-trion annihilation in monolayer WS$_2$", "authors": [ "Suman Chatterjee", "Garima Gupta", "Sarthak Das", "Kenji Watanabe", "Takashi Taniguchi", "Kausik Majumdar" ], "journal": "Phys. Rev. B 105, L121409, 2022", "doi": "10.1103/PhysRevB.105.L121409", "categories": [ "cond-mat.mes-hall", "cond-mat.mtrl-sci", "physics.app-ph", "physics.optics" ], "abstract": "Strong Coulomb interaction in monolayer transition metal dichalcogenides can facilitate nontrivial many-body effects among excitonic complexes. Many-body effects like exciton-exciton annihilation (EEA) have been widely explored in this material system. However, a similar effect for charged excitons (or trions), that is, trion-trion annihilation (TTA), is expected to be relatively suppressed due to repulsive like-charges, and has not been hitherto observed in such layered semiconductors. By a gate-dependent tuning of the spectral overlap between the trion and the charged biexciton through an \"anti-crossing\"-like behaviour in monolayer WS$_2$, here we present an experimental observation of an anomalous suppression of the trion emission intensity with an increase in gate voltage. The results strongly correlate with time-resolved measurements, and are inferred as a direct evidence of a nontrivial TTA resulting from non-radiative Auger recombination of a bright trion, and the corresponding energy resonantly promoting a dark trion to a charged biexciton state. The extracted Auger coefficient for the process is found to be tunable ten-fold through a gate-dependent tuning of the spectral overlap.", "revisions": [ { "version": "v1", "updated": "2022-04-03T08:19:56.000Z" } ], "analyses": { "keywords": [ "monolayer ws", "trion-trion annihilation", "monolayer transition metal dichalcogenides", "spectral overlap", "facilitate nontrivial many-body effects" ], "tags": [ "journal article" ], "publication": { "publisher": "APS" }, "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }