{ "id": "2107.03192", "version": "v1", "published": "2021-07-07T13:05:47.000Z", "updated": "2021-07-07T13:05:47.000Z", "title": "A hole-Cr$^{+}$ nano-magnet in a semiconductor quantum dot", "authors": [ "V. Tiwari", "M. Arino", "S. Gupta", "M. Morita", "T. Inoue", "D. Caliste", "P. Pochet", "H. Boukari", "S. Kuroda", "L. Besombes" ], "categories": [ "cond-mat.mes-hall", "quant-ph" ], "abstract": "We study a new diluted magnetic semiconductor system based on the spin of the ionized acceptor Cr$^+$. We show that the negatively charged Cr$^+$ ion, an excited state of the Cr in II-VI semiconductor, can be stable when inserted in a CdTe quantum dot (QD). The Cr$^+$ attracts a heavy-hole in the QD and form a stable hole-Cr$^+$ complex. Optical probing of this system reveals a ferromagnetic coupling between heavy-holes and Cr$^+$ spins. At low temperature, the thermalization on the ground state of the hole-Cr$^+$ system with parallel spins prevents the optical recombination of the excess electron on the 3$d$ shell of the atom. We study the dynamics of the nano-magnet formed by the hole-Cr$^+$ exchange interaction. The ferromagnetic ground states with M$_z$=$\\pm$4 can be controlled by resonant optical pumping and a spin relaxation time in the 20 $\\mu$s range is obtained at T=4.2 K. This spin memory at zero magnetic field is limited by the interaction with phonons.", "revisions": [ { "version": "v1", "updated": "2021-07-07T13:05:47.000Z" } ], "analyses": { "keywords": [ "semiconductor quantum dot", "nano-magnet", "zero magnetic field", "spin relaxation time", "ferromagnetic ground states" ], "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }