{ "id": "2102.06370", "version": "v1", "published": "2021-02-12T07:18:49.000Z", "updated": "2021-02-12T07:18:49.000Z", "title": "Accurate Extraction of Schottky Barrier Height and Universality of Fermi Level De-pinning of van der Waals Contacts", "authors": [ "Krishna Murali", "Medha Dandu", "Kenji Watanabe", "Takashi Taniguchi", "Kausik Majumdar" ], "journal": "Advanced Functional Materials, 2021", "doi": "10.1002/adfm.202010513", "categories": [ "cond-mat.mes-hall", "cond-mat.mtrl-sci", "physics.app-ph" ], "abstract": "Due to Fermi level pinning (FLP), metal-semiconductor contact interfaces result in a Schottky barrier height (SBH), which is usually difficult to tune. This makes it challenging to efficiently inject both electrons and holes using the same metal - an essential requirement for several applications, including light-emitting devices and complementary logic. Interestingly, modulating the SBH in the Schottky-Mott limit of de-pinned van der Waals (vdW) contacts becomes possible. However, accurate extraction of the SBH is essential to exploit such contacts to their full potential. In this work, we propose a simple technique to accurately estimate the SBH at the vdW contact interfaces by circumventing several ambiguities associated with SBH extraction. Using this technique on several vdW contacts, including metallic 2H-TaSe$_2$, semi-metallic graphene, and degenerately doped semiconducting SnSe$_2$, we demonstrate that vdW contacts exhibit a universal de-pinned nature. Superior ambipolar carrier injection properties of vdW contacts are demonstrated (with Au contact as a reference) in two applications, namely, (a) pulsed electroluminescence from monolayer WS$_2$ using few-layer graphene (FLG) contact, and (b) efficient carrier injection to WS$_2$ and WSe$_2$ channels in both nFET and pFET modes using 2H-TaSe$_2$ contact.", "revisions": [ { "version": "v1", "updated": "2021-02-12T07:18:49.000Z" } ], "analyses": { "keywords": [ "van der waals contacts", "schottky barrier height", "accurate extraction", "fermi level de-pinning", "vdw contact" ], "tags": [ "journal article" ], "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }