{ "id": "2101.09946", "version": "v1", "published": "2021-01-25T08:19:20.000Z", "updated": "2021-01-25T08:19:20.000Z", "title": "Determining the Proximity Effect Induced Magnetic Moment in Graphene by Polarised Neutron Reflectivity and X-ray Magnetic Circular Dichroism", "authors": [ "R. O. M. Aboljadayel", "D. M. Love", "C. A. F. Vaz", "R. S. Weatherup", "P. Braeuninger-Weimer", "M. -B. Martin", "A. Cabrero-Vilatela", "A. Ionescu", "C. J. Kinane", "T. R. Charlton", "J. Llandro", "P. M. S. Monteiro", "C. H. W. Barnes", "S. Hofmann", "S. Langridge" ], "comment": "30 pages, 13 figures", "categories": [ "cond-mat.mes-hall" ], "abstract": "We report the magnitude of the induced magnetic moment in CVD-grown epitaxial and rotated-domain graphene as a result of the proximity effect in the vicinity of the ferromagnetic substrates Co and Ni, using polarised neutron reflectivity (PNR). Although rotated-domain graphene is known to interact weakly with the ferromagnetic underlayer in comparison with the epitaxial graphene, the PNR results indicate an induced magnetic moment of $\\sim$ 0.57 $\\mu_\\textrm{B}$/C atom at 10 K for both structures. The origin of the induced magnetic moment is found to be due to the opening of the graphene's Dirac cone as a result of the strong C $p_z-3d$ hybridisation, which was confirmed by additional PNR measurements using a non-magnetic Ni$_9$Mo$_1$ and Cu substrates. We validated our PNR fitting models using the Bayesian uncertainty analysis and corroborated the results by X-ray magnetic circular dichroism measurements.", "revisions": [ { "version": "v1", "updated": "2021-01-25T08:19:20.000Z" } ], "analyses": { "keywords": [ "x-ray magnetic circular dichroism", "proximity effect induced magnetic moment", "polarised neutron reflectivity", "magnetic circular dichroism measurements" ], "note": { "typesetting": "TeX", "pages": 30, "language": "en", "license": "arXiv", "status": "editable" } } }