{ "id": "2011.12741", "version": "v1", "published": "2020-11-25T13:52:16.000Z", "updated": "2020-11-25T13:52:16.000Z", "title": "Higher-order correlations in transition metal dichalcogenides", "authors": [ "A. Kudlis", "I. Iorsh" ], "categories": [ "cond-mat.mes-hall" ], "abstract": "We analyze the many-particle correlations that affect the optical properties of transition-metal dichalcogenide monolayers. These correlations manifest themselves through the specific optical resonances such as excitons, trions, etc. As the starting point the conventional electron-hole Hamiltonian with potential in the Keldysh-Rytova form is considered. By means of this model and microscopic Heisenberg equation of motion the infinite hierarchy of differential equations can be obtained. In order to decouple a such system we address the cluster expansion technique which provides a regular procedure of consistent accounting of many-particle correlation contributions into the interband polarization dynamics. In particular, the partially taken into account three-particle correlations modify the behavior of absorption spectra with the emergence of a trion-like peak additional to excitonic ones.", "revisions": [ { "version": "v1", "updated": "2020-11-25T13:52:16.000Z" } ], "analyses": { "keywords": [ "transition metal dichalcogenides", "higher-order correlations", "microscopic heisenberg equation", "many-particle correlation contributions", "transition-metal dichalcogenide monolayers" ], "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }