{ "id": "1911.07639", "version": "v1", "published": "2019-11-18T13:52:02.000Z", "updated": "2019-11-18T13:52:02.000Z", "title": "Influence of non-equilibrium phonons on the spin dynamics of a single Cr atom", "authors": [ "V. Tiwari", "K. Makita", "M. Arino", "M. Morita", "S. Kuroda", "H. Boukari", "L. Besombes" ], "categories": [ "cond-mat.mes-hall" ], "abstract": "We analyse the influence of optically generated non-equilibrium phonons on the spin relaxation and effective spin temperature of an individual Cr atom inserted in a quantum dot. Using a three pulses pump-probe technique, we show that the spin relaxation measured in resonant optical pumping experiments strongly depends on the optical excitation conditions. We observe for an isolated Cr in the dark a heating time shorter than a few hundreds $ns$ after an initial high power non-resonant excitation pulse. A cooling time larger than a few tens of $\\mu s$, independent on the excitation, is obtained in the same experimental conditions. We show that a tunable spin-lattice coupling dependent on the density of non-equilibrium phonons can explain the observed dynamics. Low energy excitation conditions are found where the Cr spin states S$_z$=$\\pm$1 can be efficiently populated by a non-resonant optical excitation, prepared and read-out by resonant optical pumping and conserved in the dark during a few $\\mu$s.", "revisions": [ { "version": "v1", "updated": "2019-11-18T13:52:02.000Z" } ], "analyses": { "keywords": [ "non-equilibrium phonons", "single cr atom", "spin dynamics", "initial high power non-resonant excitation", "high power non-resonant excitation pulse" ], "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }