{ "id": "1904.04711", "version": "v1", "published": "2019-04-09T14:46:49.000Z", "updated": "2019-04-09T14:46:49.000Z", "title": "Phonon-assisted Photoluminescence from Dark Excitons in Monolayers of Transition Metal Dichalcogenides", "authors": [ "Samuel Brem", "August Ekman", "Dominik Christiansen", "Florian Katsch", "Malte Selig", "Cedric Robert", "Xavier Marie", "Bernhard Urbaszek", "Andreas Knorr", "Ermin Malic" ], "categories": [ "cond-mat.mes-hall", "cond-mat.mtrl-sci" ], "abstract": "The photoluminescence (PL) spectrum of transition metal dichalcogenides (TMDs) shows a multitude of emission peaks below the bright exciton line and not all of them have been explained yet. Here, we study the emission traces of phonon-assisted recombinations of momentum-dark excitons. To this end, we develop a microscopic theory describing simultaneous exciton, phonon and photon interaction and including consistent many-particle dephasing. We explain the drastically different PL below the bright exciton in tungsten- and molybdenum-based materials as result of different configurations of bright and dark states. In good agreement with experiments, we show that WSe$_2$ exhibits clearly visible low-temperature PL signals stemming from the phonon-assisted recombination of momentum-dark excitons.", "revisions": [ { "version": "v1", "updated": "2019-04-09T14:46:49.000Z" } ], "analyses": { "keywords": [ "transition metal dichalcogenides", "phonon-assisted photoluminescence", "visible low-temperature pl signals", "low-temperature pl signals stemming", "bright exciton" ], "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }