{ "id": "1902.10145", "version": "v1", "published": "2019-02-26T19:00:01.000Z", "updated": "2019-02-26T19:00:01.000Z", "title": "Correlations between Optical Properties and Voronoi-Cell Area of Quantum Dots", "authors": [ "Matthias C. Löbl", "Liang Zhai", "Jan-Philipp Jahn", "Julian Ritzmann", "Yongheng Huo", "Andreas D. Wieck", "Oliver G. Schmidt", "Arne Ludwig", "Armando Rastelli", "Richard J. Warburton" ], "categories": [ "cond-mat.mes-hall", "cond-mat.mtrl-sci" ], "abstract": "Semiconductor quantum dots (QDs) have been established as excellent photon emitters during the last decade. A QD can generate highly indistinguishable single-photons at a high rate. For application in quantum communication and integration in hybrid systems, control of the QD optical properties is essential. Understanding the connection between the optical properties of a QD and the growth process is therefore important. Here, we show for GaAs QDs, grown by infilling droplet-etched nano-holes, that the emission wavelength, neutral-to-charged exciton splitting, and diamagnetic shift are strongly correlated with the capture zone-area, an important concept from nucleation theory. Our analysis relies on photoluminescence-imaging and post-experiment determination of the QD-positions and the associated Voronoi-cells. The experiments show that the capture-zone model applies to the growth of this system even in the limit of a low QD-density in which Al-atoms diffuse over micrometer distances. The strong correlations between the various QD parameters facilitate preselection of QDs for applications with specific requirements on the QD properties; they also suggest that a narrowed QD distribution will result if QD growth on a regular lattice can be achieved.", "revisions": [ { "version": "v1", "updated": "2019-02-26T19:00:01.000Z" } ], "analyses": { "keywords": [ "voronoi-cell area", "correlations", "qd parameters facilitate preselection", "semiconductor quantum dots", "capture-zone model applies" ], "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }