{ "id": "1808.07527", "version": "v1", "published": "2018-08-22T19:09:10.000Z", "updated": "2018-08-22T19:09:10.000Z", "title": "Dephasing of InAs quantum dot p-shell excitons using two-dimensional coherent spectroscopy", "authors": [ "Takeshi Suzuki", "Rohan Singh", "Galan Moody", "Marc Aßmann", "Manfred Bayer", "Arne Ludwig", "Andreas D. Wieck", "and Steven T. Cundiff" ], "categories": [ "cond-mat.mes-hall" ], "abstract": "The dephasing mechanisms of p-shell and s-shell excitons in an InAs self-assembled quantum dot ensemble are examined using two-dimensional coherent spectroscopy (2DCS). 2DCS provides a comprehensive picture of how the energy level structure of dots affects the exciton dephasing rates and recombination lifetimes. We find that at low temperatures, dephasing of s-shell excitons is lifetime limited, whereas p-shell excitons exhibit significant pure dephasing due to scattering between degenerate spin states. At elevated temperatures, quadratic exciton-phonon coupling plays an important role in both s-shell and p-shell exciton dephasing. We show that multiple p-shell states are also responsible for stronger phonon dephasing for these transitions", "revisions": [ { "version": "v1", "updated": "2018-08-22T19:09:10.000Z" } ], "analyses": { "keywords": [ "inas quantum dot p-shell excitons", "two-dimensional coherent spectroscopy", "self-assembled quantum dot ensemble" ], "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }