{ "id": "1703.05837", "version": "v1", "published": "2017-03-16T22:03:21.000Z", "updated": "2017-03-16T22:03:21.000Z", "title": "Length-dependent Seebeck effect in single-molecule junctions beyond linear response regime", "authors": [ "Natalya A. Zimbovskaya" ], "comment": "7 pages, 4 figures", "categories": [ "cond-mat.mes-hall" ], "abstract": "In the present work we theoretically study characteristics of nonlinear Seebeck effect in a single-molecule junction with chain-like bridge of an arbitrary length. We have employed tight-binding models to compute electron transmission trough the system. We concentrate on analysis of dependences of thermovoltage $V_{th} $ and differential thermopower $ S $ on the bridge length. It is shown that $ V_{th} $ becomes stronger and $ S $ grows as the bridge lengthens. We discuss the effects of the bridge coupling to the electrodes and of specific characteristics of terminal sites on the bridge on the length-dependent $ V_{th} $ and $ S $ which appear when the system operates beyond linear response regime.", "revisions": [ { "version": "v1", "updated": "2017-03-16T22:03:21.000Z" } ], "analyses": { "keywords": [ "linear response regime", "length-dependent seebeck effect", "single-molecule junction", "electron transmission trough", "nonlinear seebeck effect" ], "note": { "typesetting": "TeX", "pages": 7, "language": "en", "license": "arXiv", "status": "editable" } } }