{ "id": "1611.02415", "version": "v1", "published": "2016-11-08T07:39:39.000Z", "updated": "2016-11-08T07:39:39.000Z", "title": "Time-resolved spectroscopy with entangled photons", "authors": [ "Dmitry A. Kalashnikov", "Elizaveta V. Melik-Gaykazyan", "Alexey A. Kalachev", "Ye Feng Yu", "Arseniy I. Kuznetsov", "Leonid A. Krivitsky" ], "comment": "Submitted for publication", "categories": [ "quant-ph", "physics.ins-det", "physics.optics" ], "abstract": "Interaction of light with media often occurs with a femtosecond response time. Its measurement by conventional techniques requires the use of femtosecond lasers and sophisticated time-gated optical detection1-3. Here we demonstrate that by exploiting quantum interference of entangled photons it is possible to measure the phase relaxation time of a media on the femtosecond time scale (down to 100 fs) using accessible continuous wave laser and single-photon counting. We insert the sample in the Hong-Ou-Mandel interferometer4 and infer the phase relaxation time from the modification of the two-photon interference pattern. In addition to its simplicity and ease of use, the technique does not require compensation of group velocity dispersion5-8 and does not induce photo-damage of the samples. This technique will be useful for characterization of ultrafast phase relaxation processes in material science, chemistry, and biology.", "revisions": [ { "version": "v1", "updated": "2016-11-08T07:39:39.000Z" } ], "analyses": { "keywords": [ "entangled photons", "time-resolved spectroscopy", "phase relaxation time", "ultrafast phase relaxation processes", "femtosecond response time" ], "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }