{ "id": "1609.08773", "version": "v1", "published": "2016-09-28T05:09:30.000Z", "updated": "2016-09-28T05:09:30.000Z", "title": "Beyond the effective mass approximation: predictive theory of the nonlinear optical response of conduction electrons", "authors": [ "Shukai Yu", "Kate H. Heffernan", "Diyar Talbayev" ], "categories": [ "cond-mat.mes-hall", "physics.optics" ], "abstract": "We present an experimental and computational study of the nonlinear optical response of conduction electrons to intense terahertz (THz) electric field. Our observations (saturable absorption and an amplitude-dependent group refractive index) can be understood on the qualitative level as the breakdown of the effective mass approximation. However, a predictive theoretical description of the nonlinearity has been missing. We propose a model based on the semiclassical electron dynamics, a realistic band structure, and the free electron Drude parameters to accurately calculate the experimental observables in InSb. Our results open a path to predictive modeling of the conduction-electron optical nonlinearity in semiconductors, metamaterials, as well as high-field effects in THz plasmonics.", "revisions": [ { "version": "v1", "updated": "2016-09-28T05:09:30.000Z" } ], "analyses": { "keywords": [ "nonlinear optical response", "effective mass approximation", "conduction electrons", "predictive theory", "free electron drude parameters" ], "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }