{ "id": "1603.06027", "version": "v1", "published": "2016-03-19T01:06:59.000Z", "updated": "2016-03-19T01:06:59.000Z", "title": "First-principles study of the terahertz third-order nonlinear response of metallic armchair graphene nanoribbons", "authors": [ "Yichao Wang", "David R. Andersen" ], "categories": [ "cond-mat.mes-hall" ], "abstract": "We compute the terahertz third-order nonlinear conductance of metallic armchair graphene nanoribbons using time-dependent perturbation theory. Significant enhancement of the intrinsic nonlinear third-order conductance over the result for intrinsic 2D single-layer graphene is observed over a wide range of temperatures and sample geometries. We also investigate the nonlinear response of extrinsic metallic acGNR with |Ef| much smaller than 200 meV. We find that the third-order conductance exhibits a strong Fermi level dependence at low temperatures. A third-order critical field strength of between roughly 1 and 5 kV/m is computed for the nonlinear Kerr terms as a function of temperature. For the third-harmonic terms, the minimum critical field is computed to be around 5 kV/m.", "revisions": [ { "version": "v1", "updated": "2016-03-19T01:06:59.000Z" } ], "analyses": { "keywords": [ "metallic armchair graphene nanoribbons", "terahertz third-order nonlinear response", "first-principles study", "terahertz third-order nonlinear conductance", "intrinsic 2d single-layer graphene" ], "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable", "adsabs": "2016arXiv160306027W" } } }