{ "id": "1502.05964", "version": "v1", "published": "2015-02-20T18:23:29.000Z", "updated": "2015-02-20T18:23:29.000Z", "title": "Influences of Exciton Diffusion and Exciton-Exciton Annihilation on Photon Emission Statistics of Carbon Nanotubes", "authors": [ "Xuedan Ma", "Oleskiy Roslyak", "Juan G. Duque", "Xiaoying Pang", "Stephen K. Doorn", "Andrei Piryatinski", "David H. Dunlap", "Han Htoon" ], "comment": "15 pages, 4 figures", "categories": [ "cond-mat.mes-hall" ], "abstract": "Pump-dependent photoluminescence imaging and 2nd order photon correlation studies have been performed on individual single-walled carbon nanotubes (SWCNTs) at room temperature that enable the extraction of both the exciton diffusion constant and the Auger recombination coefficient. A linear correlation between these is attributed to the effect of environmental disorder in setting the exciton mean free-path and capture-limited Auger recombination at this lengthscale. A suppression of photon antibunching is attributed to creation of multiple spatially non-overlapping excitons in SWCNTs whose diffusion length is shorter than the laser spot size. We conclude that complete antibunching at room temperature requires an enhancement of exciton-exciton annihilation rate that may become realizable in SWCNTs allowing for strong exciton localization.", "revisions": [ { "version": "v1", "updated": "2015-02-20T18:23:29.000Z" } ], "analyses": { "keywords": [ "photon emission statistics", "exciton-exciton annihilation", "carbon nanotubes", "exciton diffusion", "2nd order photon correlation studies" ], "note": { "typesetting": "TeX", "pages": 15, "language": "en", "license": "arXiv", "status": "editable" } } }