{ "id": "1408.5263", "version": "v1", "published": "2014-08-22T10:58:10.000Z", "updated": "2014-08-22T10:58:10.000Z", "title": "Stacking faults as quantum wells in nanowires: Density of states, oscillator strength and radiative efficiency", "authors": [ "P. Corfdir", "C. Hauswald", "J. K. Zettler", "T. Flissikowski", "J. Lähnemann", "S. Fernández-Garrido", "L. Geelhaar", "H. T. Grahn", "O. Brandt" ], "categories": [ "cond-mat.mes-hall" ], "abstract": "We investigate the nature of excitons bound to I1 basal-plane stacking faults [(I1;X)] in GaN nanowire ensembles by continuous-wave and time-resolved photoluminescence spectroscopy. Based on the linear increase of the radiative lifetime of these excitons with temperature, they are demonstrated to exhibit a two-dimensional density of states, i. e., a basal-plane stacking fault acts as a quantum well. From the slope of the linear increase, we determine the oscillator strength of the (I1;X) and show that the value obtained reflects the presence of large internal electrostatic fields across the stacking fault. While the recombination of donor-bound and free excitons in the GaN nanowire ensemble is dominated by nonradiative phenonema already at 10 K, we observe that the (I1;X) recombines purely radiatively up to 60 K. This finding provides important insight into the nonradiative recombination processes in GaN nanowires. First, the radiative lifetime of about 6 ns measured at 60 K sets an upper limit for the surface recombination velocity of 450 cm/s considering the nanowires mean diameter of 105 nm. Second, the density of nonradiative centers responsible for the fast decay of donor-bound and free excitons cannot be higher than 2x10^16 cm^-3. As a consequence, the nonradiative decay of donor-bound excitons in these GaN nanowire ensembles has to occur indirectly via the free exciton state.", "revisions": [ { "version": "v1", "updated": "2014-08-22T10:58:10.000Z" } ], "analyses": { "subjects": [ "78.67.Uh", "71.35.-y", "71.55.Eq", "78.47.jd" ], "keywords": [ "oscillator strength", "quantum wells", "radiative efficiency", "gan nanowire ensemble", "free exciton" ], "tags": [ "journal article" ], "publication": { "doi": "10.1103/PhysRevB.90.195309", "journal": "Physical Review B", "year": 2014, "month": "Nov", "volume": 90, "number": 19, "pages": 195309 }, "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable", "adsabs": "2014PhRvB..90s5309C" } } }