{ "id": "1408.0672", "version": "v2", "published": "2014-08-04T13:09:09.000Z", "updated": "2014-08-06T11:17:07.000Z", "title": "Origin of coherent G band phonon spectra in single wall carbon nanotubes", "authors": [ "A. R. T. Nugraha", "E. H. Hasdeo", "G. D. Sanders", "C. J. Stanton", "R. Saito" ], "comment": "submitted to Phys. Rev. B", "categories": [ "cond-mat.mes-hall" ], "abstract": "Coherent phonons in single wall carbon nanotubes (SWNTs) are observed as oscillations of the differential absorption coefficient as a function of time by means of pump-probe spectroscopy. For the radial breathing mode (RBM) of a SWNT, the coherent phonon signal is understood to be a result of the modulated diameter-dependent energy gaps due to the coherent RBM phonon oscillations. However, this mechanism might not be the dominant contribution to other phonon modes in the SWNT. In particular, for the G band phonons, which correspond to bond-stretching motions, we find that the modulation of the interatomic dipole matrix element gives rise to a strong coherent G band phonon intensity comparable to the coherent RBM phonon intensity. We also further discuss the dependence of coherent G band and RBM phonon amplitudes on the laser excitation pulse width.", "revisions": [ { "version": "v2", "updated": "2014-08-06T11:17:07.000Z" } ], "analyses": { "subjects": [ "78.67.Ch", "78.47.J-", "73.22.-f", "63.22.Gh" ], "keywords": [ "single wall carbon nanotubes", "band phonon spectra", "coherent rbm phonon intensity", "coherent phonon", "laser excitation pulse width" ], "tags": [ "journal article" ], "publication": { "doi": "10.1103/PhysRevB.91.045406", "journal": "Physical Review B", "year": 2015, "month": "Jan", "volume": 91, "number": 4, "pages": "045406" }, "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable", "adsabs": "2015PhRvB..91d5406N" } } }