{ "id": "1005.4069", "version": "v2", "published": "2010-05-21T20:19:22.000Z", "updated": "2010-09-22T16:18:18.000Z", "title": "Quantum simulation of multiple-exciton generation in a nanocrystal by a single photon", "authors": [ "Wayne M. Witzel", "Andrew Shabaev", "C. Stephen Hellberg", "Verne L. Jacobs", "Alexander L. Efros" ], "journal": "Phys. Rev. Lett. 105, 137401 (2010)", "doi": "10.1103/PhysRevLett.105.137401", "categories": [ "cond-mat.mes-hall", "cond-mat.str-el" ], "abstract": "We have shown theoretically that efficient multiple exciton generation (MEG) by a single photon can be observed in small nanocrystals (NCs). Our quantum simulations that include hundreds of thousands of exciton and multi-exciton states demonstrate that the complex time-dependent dynamics of these states in a closed electronic system yields a saturated MEG effect on a picosecond timescale. Including phonon relaxation confirms that efficient MEG requires the exciton--biexciton coupling time to be faster than exciton relaxation time.", "revisions": [ { "version": "v2", "updated": "2010-09-22T16:18:18.000Z" } ], "analyses": { "subjects": [ "78.67.Bf", "73.21.La", "78.47.-p", "78.67.Hc" ], "keywords": [ "single photon", "quantum simulation", "multiple-exciton generation", "efficient multiple exciton generation", "exciton relaxation time" ], "tags": [ "journal article" ], "publication": { "publisher": "APS", "journal": "Physical Review Letters", "year": 2010, "month": "Sep", "volume": 105, "number": 13, "pages": 137401 }, "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable", "adsabs": "2010PhRvL.105m7401W" } } }