{ "id": "1001.4546", "version": "v1", "published": "2010-01-25T21:31:36.000Z", "updated": "2010-01-25T21:31:36.000Z", "title": "Excitons and high-order optical transitions in individual carbon nanotubes", "authors": [ "Stephane Berciaud", "Christophe Voisin", "Hugen Yan", "Bhupesh Chandra", "Robert Caldwell", "Yuyao Shan", "Louis E. Brus", "James Hone", "Tony F. Heinz" ], "journal": "Phys. Rev. B 81, 041414(R) (2010)", "doi": "10.1103/PhysRevB.81.041414", "categories": [ "cond-mat.mes-hall" ], "abstract": "We examine the excitonic nature of high-lying optical transitions in single-walled carbon nanotubes by means of Rayleigh scattering spectroscopy. A careful analysis of the principal transitions of individual semiconducting and metallic nanotubes reveals that in both cases the lineshape is consistent with an excitonic model, but not one of free-carriers. For semiconducting species, side-bands are observed at ~200 meV above the third and fourth optical transitions. These features are ascribed to exciton-phonon bound states. Such side-bands are not apparent for metallic nanotubes,as expected from the reduced strength of excitonic interactions in these systems.", "revisions": [ { "version": "v1", "updated": "2010-01-25T21:31:36.000Z" } ], "analyses": { "keywords": [ "individual carbon nanotubes", "high-order optical transitions", "metallic nanotubes", "exciton-phonon bound states", "single-walled carbon nanotubes" ], "tags": [ "journal article" ], "publication": { "publisher": "APS", "journal": "Phys. Rev. B" }, "note": { "typesetting": "TeX", "pages": 0, "language": "en", "license": "arXiv", "status": "editable" } } }